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De Niro all day on this. And yeah you left out Casino and a Bronx tale...but I guess you could argue he didn't play gangsters in those
Robert DeNiro*Only Films where the actor played a gangster in the film*
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The Godfather
The Godfather II
Scarface
Carlito's Way
Donnie Brasco
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The Godfather II
Goodfellas
Heat
Once Upon A Time in America
The Untouchables
Plus of course Pacino was in Heat.Casino!?!?